DNA brick crystals with prescribed depths

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DNA brick crystals with prescribed depths.

The ability to assemble functional materials with precise spatial arrangements is important for applications ranging from protein crystallography to photovoltaics. Here, we describe a general framework for constructing two-dimensional crystals with prescribed depths and sophisticated three-dimensional features. The crystals are self-assembled from single-stranded DNA components called DNA brick...

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DNA Brick Crystals with Prescribed Depth

We describe a general framework for constructing two-dimensional crystals with prescribed depth and sophisticated three-dimensional features. These crystals may serve as scaffolds for the precise spatial arrangements of functional materials for diverse applications. The crystals are selfassembled from single-stranded DNA components called DNA bricks. We demonstrate the experimental construction...

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DNA brick self-assembly with an off-lattice potential.

We report Monte Carlo simulations of a simple off-lattice patchy-particle model for DNA 'bricks'. We relate the parameters that characterise this model with the binding free energy of pairs of single-stranded DNA molecules. We verify that an off-lattice potential parameterised in this way reproduces much of the behaviour seen with a simpler lattice model we introduced previously, although the r...

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The observation by Ke et al. [Science 338, 1177 (2012)] that large numbers of short, predesigned DNA strands can assemble into three-dimensional target structures came as a great surprise, as no colloidal self-assembling system has ever achieved the same degree of complexity. That failure seemed easy to rationalize: the larger the number of distinct building blocks, the higher the expected erro...

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ژورنال

عنوان ژورنال: Nature Chemistry

سال: 2014

ISSN: 1755-4330,1755-4349

DOI: 10.1038/nchem.2083